Syntheses of Coniine, DAB-1, and Nectrisine

Untitled Tot_Syn_Style-1

Our work on the total syntheses of the alkaloid natural products (–)-coniine, DAB-1, and nectrisine just appeared in ACS Omega! This was collaborative work with Prof. Deardorff to develop a robust synthesis of these biologically active natural products. The approach utilizes an enzyme-catalyzed hydrocyanation to establish the key stereochemistry, which is followed by transition metal-catalyzed reactions to transform this building block into the natural products. We envision this approach as a general platform for the enantioselective syntheses of alkaloid natural products. Congrats to the undergraduates that worked on this project together!

Leave a Reply

Fill in your details below or click an icon to log in:

WordPress.com Logo

You are commenting using your WordPress.com account. Log Out /  Change )

Facebook photo

You are commenting using your Facebook account. Log Out /  Change )

Connecting to %s